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Third harmonic generation (THG) in dielectric films with femtosecond laser pulses is used to study properties of dielectric thin films and stacks thereof below and above the 1-on-1 laser damage threshold. Deviations from the ideal cubic relationship between third-harmonic signal and incident fundamental fluence are a result of several fundamental processes. Their relative contributions are assessed by comparing results from LIDT and conversion efficiency measurements as well as beam profile and pump-probe studies.
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Amir Khabbazi Oskouei, Luke Emmert, Morten Steinecke, Marco Jupé, Detlev Ristau, Lars Jensen, Wolfgang Rudolph, "Third harmonic (TH) generation: a tool to study dielectric material properties near the laser induced damage threshold (LIDT)," Proc. SPIE 11173, Laser-induced Damage in Optical Materials 2019, 111731L (20 November 2019); https://doi.org/10.1117/12.2536440