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We present time resolved measurements on low dimensional nanomaterials like individual (6,4) single-walled carbon nanotubes and monolayers of MoSe2 via transient interferometric scattering (TiSCAT) microscopy. For this a novel fiber laser system was developed comprising a tunable probe arm and low noise performance. The sensitivity of the measurement is demonstrated for very low excitation powers to prevent photodamage of the sample. Signal variations close to the shot-noise limit can be resolved even with low excitation powers in the order of 1 μW. In combination with the tunability of the laser system the absorption spectrum of a single SWCNT was determined.
Konrad Birkmeier,Andreas Brodschelm,Florian Tauser,Reto Häring,Bernhard Wolfring, andAchim Hartschuh
"Transient interferometric scattering microscopy on nanoscale objects with high sensitivity", Proc. SPIE 12410, Nanoscale and Quantum Materials: From Synthesis and Laser Processing to Applications 2023, 1241009 (15 March 2023); https://doi.org/10.1117/12.2668432
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Konrad Birkmeier, Andreas Brodschelm, Florian Tauser, Reto Häring, Bernhard Wolfring, Achim Hartschuh, "Transient interferometric scattering microscopy on nanoscale objects with high sensitivity," Proc. SPIE 12410, Nanoscale and Quantum Materials: From Synthesis and Laser Processing to Applications 2023, 1241009 (15 March 2023); https://doi.org/10.1117/12.2668432