Paper
10 July 2007 The possibility of single-shot high-resolution CARS lineshape spectroscopy
K. A. Vereschagin, A. K. Vereschagin
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Abstract
Influence of a random nature of light on a possibility of realization of single-shot high-resolution lineshape spectroscopy is discussed. Non-linear interaction of light with matter in CARS process could change initial light statistics. Broad band CARS with use of conventional dye lasers as a source of Stokes waves conserves the initial <<exponential>> light statistics peculiar to broadband radiation with modes structure. Dual Broad Band CARS-approach can change light statistics from <<exponential>> in Stokes wave to <<normal>> in anti-Stokes radiation providing the possibility to realize the single-shot high-resolution lineshape spectroscopy.
© (2007) COPYRIGHT Society of Photo-Optical Instrumentation Engineers (SPIE). Downloading of the abstract is permitted for personal use only.
K. A. Vereschagin and A. K. Vereschagin "The possibility of single-shot high-resolution CARS lineshape spectroscopy", Proc. SPIE 6727, ICONO 2007: Nonlinear Laser Spectroscopy and High-Precision Measurements; and Fundamentals of Laser Chemistry and Biophotonics, 67271K (10 July 2007); https://doi.org/10.1117/12.752376
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KEYWORDS
Convolution

Spectroscopy

Dye lasers

Raman spectroscopy

Laser scattering

Statistical analysis

Spectral resolution

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