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Multicolor visible light emitting NIR-excited Tm/Ho/Yb-codoped tantalum oxide nanopowders were produced using the
sol-gel method. The generation of wide color gamut fluorescence in glass-ceramic with orthorhombic Ta2O5
nanocrystals dispersed into amorphous silica-based matrix is observed. The light emission spectroscopic properties of
the rare-earth doped SiO2:Ta2O5 nanocomposites as a function of the tantalum content and temperature of annealing is
examined. Simultaneously emitted multicolor fluorescence consisting of blue(480 nm), green(540 nm) and red(650 nm)
upconversion signals in the SiO2:Ta2O5 system doped with holmium and thulium and sensitized with ytterbium, is
demonstrated. It is also demonstrated that the proper choice of the rare-earth content and the NIR excitation power
yielded the generation and control of the three primary colors and allows the emission of a balanced white overall
luminescence from the glass-ceramic nanopowder samples.
Artur S. Gouveia-Neto,Luciano A. Bueno,Ernande B. Costa,Elias A. Silva Jr.,Jefferson L. Ferrari,Karmel O. Lima, andRogéria R. Gonçalves
"Generation of wide color gamut visible light in NIR-excited thulium-holmium-ytterbium codoped tantalum oxide nanopowders", Proc. SPIE 7598, Optical Components and Materials VII, 759806 (25 February 2010); https://doi.org/10.1117/12.838866
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Artur S. Gouveia-Neto, Luciano A. Bueno, Ernande B. Costa, Elias A. Silva Jr., Jefferson L. Ferrari, Karmel O. Lima, Rogéria R. Gonçalves, "Generation of wide color gamut visible light in NIR-excited thulium-holmium-ytterbium codoped tantalum oxide nanopowders," Proc. SPIE 7598, Optical Components and Materials VII, 759806 (25 February 2010); https://doi.org/10.1117/12.838866