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Layer-thickness dependence of Si-nanocrystal (Si-NC) formation induced by furnace annealing in amorphous Si (a-Si)
/SiO2 multilayers is experimentally demonstrated with a radio-frequency-sputtered sample that has a-Si layers with
different thicknesses. Further, a modified model is developed to explain the Si-NC formation based on the Gibbs free
energy variation and it takes into account the whole formation process including nucleation and following growth. The
theoretical results show that there is a lower limit of Si layer thickness below which the crystal formation cannot occur
for a-Si/SiO2 multilayers, and the oxide interfaces cannot constrain the lateral growth of Si-NCs, which may lead to their
touches within the Si layers.
Keyong Chen,Xue Feng, andYidong Huang
"Layer-thickness-dependent formation of Si-nanocrystals embedded in
amorphous Si/SiO2 multilayers", Proc. SPIE 7991, Display, Solid-State Lighting, Photovoltaics, and Optoelectronics in Energy II, 799102 (11 January 2011); https://doi.org/10.1117/12.888342
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Keyong Chen, Xue Feng, Yidong Huang, "Layer-thickness-dependent formation of Si-nanocrystals embedded in amorphous Si/SiO2 multilayers," Proc. SPIE 7991, Display, Solid-State Lighting, Photovoltaics, and Optoelectronics in Energy II, 799102 (11 January 2011); https://doi.org/10.1117/12.888342