In this paper we tell the story of the X-ray laser, which began as an attempt to extend optical lasers to shorter wavelengths in the 1970’s. Research took off in the 1980’s driven by the rivalry between the United States and Soviet Union in their quest to create a “Star Wars” laser shield against ICBM’s. At the same time large inertial fusion confinement (ICF) lasers, such as Novette and Nova at LLNL, were able to create the first laboratory X-ray lasers in Ne-like Se at 20.6 and 20.9 nm using 2 kJ of energy in a 0.5 ns pulse. These large ICF lasers could only be fired every few hours and used very thin expensive exploding foils as the targets. With the demonstration of the pre-pulse technique at Nova, where a small pulse of a few joules heated a solid target and create a pre-plasma that was then be heated by a second large pulse to create the lasing conditions, X-ray lasers started working robustly at many laser facilities around the world. The advent of high repetition rate psec lasers combined with the pre-pulse technique and grazing incident geometry opened the door to the many table-top X-ray lasers today which can be driven by less than 1 J of energy and operate at 100 Hz repetition rates. This has opened many new research opportunities for scientific research using X-ray lasers.
Joseph Nilsen, D. Burridge, L.M. Hobbs, D. Hoarty, P. Beiersdorfer, G. Brown, N. Hell, D. Panchenko, M. Gu, A. Saunders, H. Scott, R. London, P. Hatfield, M. Hill, L. Wilson, R. Charles, C. R. Brown, S. Rose
Many resonant photo-pumped X-ray laser schemes that use a strong pump line such as Ly-α or He-α to populate the upper laser state of a separate lasing material have been proposed over the last four decades but none have been demonstrated. As a first step to creating a photo-pumped X-ray laser we decided to reinvestigate some of these schemes at the Orion laser facility with the goal to demonstrate enhanced fluorescence as a first step toward creating a laser. In particular we look at using the Ly-α or He-α K lines to pump the 1s – 3p and 4p transitions in H-like Cl and see fluorescence on the 4f -3d line at 65 Å and the 3d – 2p line at 23 Å. Preliminary experiments are presented that show a modest enhancement of 40% on the 3d-2p line. As an alternative we also look at enhancing the 2p – 2s line in Ne-like Ge at 65Å using the Ly-α Mg line to photo-pump the 2s – 3p line of Ne-like Ge. Calculations are presented that suggest modest enhancements of 2.5 and recent experiments will be presented that show emission from a Ge plasma pumped by the Ly-α Mg line.
Six years ago an inner-shell X-ray laser was demonstrated at 849 eV in singly ionized neon using the X-FEL at 960 eV to photo-ionize the 1s electron in neutral neon followed by lasing on the 2p – 1s transition in singly-ionized neon. It required a very strong X-ray source that could photo-ionize the 1s (K-shell) electron on a time scale comparable to the intrinsic auger lifetime of 2 fsec. We extend this work from K-shell to L-shell transitions. We show how the XFEL could be used photo-ionize L-shell electrons to drive gain on n=3-2 transitions in singly-ionized Ar and Cu plasmas. For Ar this requires an XFEL above 250 or 330 eV with lasing on 3-2 lines at 220 and 310 eV. The Cu scheme requires an XFEL above 960 eV with lasing on 3d-2p lines at 928 and 948 eV. We will also discuss extending this work to photoionizing the M-shell with lasing on n=4-3 transitions in singly ionized neodymium.
Four years ago an inner-shell X-ray laser was demonstrated at 849 eV in singly ionized neon gas using the LCLS X-FEL at 960 eV to photo-ionize the 1s electron in neutral neon followed by lasing on the 2p – 1s transition in singly-ionized neon. It took many decades to demonstrate this scheme because it required a very strong X-ray source that could photo-ionize the 1s (K shell) electrons in neon on a time scale comparable to the intrinsic auger lifetime in the neon, which is typically 2 fsec. In this work we model the neon inner shell X-ray laser under similar conditions to those used at LCLS and investigate how we can improve the efficiency of the neon laser and reduce the drive requirements by tuning the XFEL to the 1s-3p transition in neutral neon in order to create gain on the 2p-1s line in neutral neon. We also explore using the XFEL to drive gain on 3-2 transitions in singly-ionized Ar and Cu plasmas.
X-ray Thomson scattering is being developed as a method to measure the temperature, electron density, and ionization
state of high energy density plasmas such as those used in inertial confinement fusion. Most experiments are currently
done at large laser facilities that can create bright X-ray sources, however the advent of the X-ray free electron laser (XFEL)
provides a new bright source to use in these experiments.One challenge with X-ray Thomson scattering
experiments is understanding how to model the scattering for partially ionized plasmas in order to include the
contributions of the bound electrons in the scattered intensity. In this work we take the existing models of Thomson
scattering that include elastic ion-ion scattering and the electron-electron plasmon scattering and add the contribution of
the bound electrons in the partially ionized plasmas. We validated our model by analyzing existing beryllium
experimental data. We then consider several higher Z materials such as Cr and predict the existence of additional peaks
in the scattering spectrum that requires new computational tools to understand. We also show examples of experiments
in CH and Al that have bound contributions that change the shape of the scattered spectra.
Nearly four decades ago H-like and He-like resonantly photo-pumped laser schemes were proposed for producing X-ray
lasers. However, demonstrating these schemes in the laboratory has proved to be elusive because of the difficulty of
finding a strong resonant pump line. With the advent of the X-ray free electron laser (X-FEL) at the SLAC Linac
Coherent Light Source (LCLS) we now have a tunable X-ray laser source that can be used to replace the pump line in
previously proposed laser schemes and allow researchers to study the physics and feasibility of resonantly photo-pumped
laser schemes. In this paper we use the X-FEL at 1174 eV to photo-pump the singly excited 1s2p state of Helike
Ne to the doubly excited 2p3p state and model gain on the 2p3p-2p2s transition at 175 eV and the 2p3p-1s3p
transition at 1017 eV. One motivation for studying this scheme is to explore possible quenching of the gain due to strong
non-linear coupling effects from the intense X-FEL beam. We compare this scheme with photo-pumping the He-like Ne
ground state to the 1s3p singly excited state followed by lasing on the 3p-2s and 3d-2p transitions at 158 and 151 eV.
Experiments are being planned at LCLS to study these laser processes and coherent quantum effects.
Nearly four decades ago H-like and He-like resonantly photo-pumped laser schemes were proposed for producing X-ray lasers. However, demonstrating these schemes in the laboratory has proved to be elusive. One challenge has been the difficulty of finding an adequate resonance between a strong pump line and a line in the laser plasma that drives the laser transition. Given a good resonance, a second challenge has been to create both the pump and laser plasma in close proximity so as to allow the pump line to transfer its energy to the laser material. With the advent of the X-FEL at LCLS we now have a tunable X-ray laser source that can be used to replace the pump line in previously proposed laser
schemes and allow researchers to study the physics and feasibility of photo-pumped laser schemes. In this paper we
model the Na-pumped Ne X-ray laser scheme that was proposed and studied many years ago by replacing the Na He-α pump line at 1127 eV with the X-FEL at LCLS. We predict gain on the 4f - 3d transition at 231 Å. We also examine the feasibility of photo-pumping He-like V and lasing on the 4f - 3d transition at 38.7 Å, which would be within the water-window. In addition we look at the possibility of photo-pumping Ne-like Fe and creating gain on the 4d - 3p transition at 53 Å and the 3p - 3s transition at 255 Å.
Soft x-ray interferometry was used to measure the evolution of dense converging plasmas created by laser irradiation of 500 μm diameter semi-cylindrical carbon targets. Optical laser pulses with an intensity of ~1×1012W cm-2 and 120 ps duration were used to heat the surface of the cavities. The dense plasma formed expands from the walls converging slightly off the semi-cylinder's axis, giving rise to a bright localized high density plasma region. A sequence of electron density maps were measure using a 46.9 nm wavelength tabletop capillary discharge soft x-ray laser probe and an amplitude division interferometer based on diffraction gratings. The measured density profiles are compared with simulations conducted using the multi-diminensional hydrodynamic code HYDRA. The benchmarked model was then used to simulate particle trajectories which reveal that the increase in electron density near the axis is mainly the result of the convergence of plasma that originated at the bottom of the groove during laser irradiation.
Over the last decade the electron density of plasmas has been measured using X-ray laser interferometers in the 14 to 47
nm wavelength regime. With the same formula used in decades of experiments with optical interferometers, the data
analysis assumes the index of refraction is due only to the free electrons, which makes the index less than one. Over the
last several years, interferometer experiments in C, Al, Ag, and Sn plasmas have observed plasmas with index of
refraction greater than one at 14 or 47 nm and demonstrated unequivocally that the usual formula for calculating the
index of refraction is not always valid as the contribution from bound electrons can dominate the free electrons in
certain cases. In this paper we search for other materials with strong anomalous dispersion that could be used in X-ray
laser interferometer experiments to help understand this phenomena. An average atom code is used to calculate the
plasma properties. This paper discusses the calculations of anomalous dispersion in Ne and Na plasmas near 47 nm and
Xe plasmas near 14 nm. With the advent of the FLASH X-ray free electron laser in Germany and the LCLS X-FEL
coming online at Stanford in 2 years the average atom code will be an invaluable tool to explore plasmas at higher X-ray
energy to identify potential experiments for the future. During the next decade X-ray free electron lasers and other
X-ray sources will be used to probe a wider variety of plasmas at higher densities and shorter wavelengths so
understanding the index of refraction in plasmas will be even more essential.
For decades the electron density of plasmas has been measured using optical interferometers. With the availability of good X-ray laser sources in the last decade interferometers have been extended into the wavelength range 14 - 47 nm, which has enabled researchers to probe even higher density plasmas. The data analysis assumes the index of refraction is due only to the free electrons, which makes the index less than one. Recent interferometer experiments in Al plasmas observed plasmas with index of refraction greater than one at 14 nm and brought into question the validity of the usual formula for calculating the index. In this paper we show how the anomalous dispersion from bound electrons can dominate the free electron contribution to the index of refraction in many plasmas and make the index greater than one or enhance the contribution to the index such that one would greatly overestimate the density of the plasma using interferometers. Using a new average-atom code we calculate the index of refraction in many plasmas at different temperatures for photon energies from 0 to 100 eV and compare against calculations done with OPAL. We also present examples of other plasmas that may have index of refraction greater than one at X-ray laser energies. During the next decade X-ray free electron lasers and other X-ray sources will be available to probe a wider variety of plasmas at higher densities and shorter wavelengths so understanding the index of refraction in plasmas will be even more essential.
We have used soft x-ray laser interferometry to study dense colliding plasmas produced by laser irradiation of semi-cylindrical targets. Results are reported on the evolution of 1 mm long plasmas created by heating 500 μm diameter half holhraum copper targets with an intensity of ~1.6 1012 W.cm-2 from 120 ps duration laser pulses of 800 nm wavelength. The setup combines a robust high throughput amplitude division interferometer based on diffraction gratings with a 46.9 nm table-top capillary discharge laser. Series of high contrast interferograms were obtained depicting the evolution of the copper plasmas into a localized plasma that reaches densities above 1×1020 cm-3 when the plasmas collide near the center of the cavity. The technique allows the generation of high resolution density maps of colliding plasma with various degree of collisionality for comparison with code simulations.
We report clear evidence of the existence of multiply ionized plasmas with index of refraction greater than one at soft x-ray wavelengths. Moreover, it is shown to be a general phenomenon affecting broad spectral regions in numerous highly ionized plasmas. The experimental evidence consists of the observation of anomalous fringe shifts in soft x-ray laser interferograms of laser-created Al plasmas probed at 14.7 nm and of Ag and Sn laser-created plasmas probed at 46.9 nm. The comparison of measured and simulated interferograms shows that these anomalous fringe shifts result from the dominant contribution of low charge ions to the index of refraction. This usually neglected bound electron contribution can affect the propagation of soft x-ray radiation in plasmas and the interferometric diagnostics of plasmas for many elements and at different wavelengths.
The absolute time of emission of the x-ray laser output with respect to the arrival of a 100-ps pump pulse has been measured with the aid of a calibrated timing fiducial. The results show the x-ray laser to appear up to 60 ps (80 ps) before the peak of the pump pulse in the case of the Sn (Pd) x-ray laser, which is in good agreement with results obtained from hydrodynamic, atomic physics, and raytracing simulations. The pulse duration was found to be ~40 ps for both the Sn and the Pd x-ray lasers.
We summarize results of several successful dense plasma diagnostics experiments realized combining two different kinds of table-top soft x-ray lasers with an amplitude division interferometer based on diffraction grating beam splitters. In the first set of experiments this robust high throughput diffraction grating interferometer (DGI) was used with a 46.9 nm portable capillary discharge laser to study the dynamics of line focus and point focus laser-created plasmas. The measured electron density profiles, which differ significantly from those expected from a classical expansion, unveil important twodimensional effects of the dynamics of these plasmas. A second DGI customized to operate in combination with a 14.7 nm Ni-like Pd transient gain laser was used to perform interferometry of line focus laser-created plasmas with picosecond time resolution. These measurements provide valuable new benchmarks for complex hydrodynamic codes and help bring new understanding of the dynamics of dense plasmas. The instrumentation and methodology we describe is scalable to significantly shorter wavelengths, and constitutes a promising scheme for extending interferometry to the study of very dense
plasmas such as those investigated for inertial confinment fusion.
We present the longitudinal coherence measurement of the transient inversion collisional x-ray laser for the first time. The Ni-like Pd x-ray laser at 14.68 nm is generated by the LLNL COMET laser facility and is operating in the gain-saturated regime. Interference fringes are produced using a Michelson interferometer setup in which a thin multilayer-coated membrane is used as a beam splitter. The longitudinal coherence length for the picosecond duration 4d1S0 -> 4p1P1 lasing transition is determined to be ~400 µm (1/e HW) by adjusting the length of one interferometer arm and measuring the resultant variation in fringe visibility. This is four times improved coherence than previous measurements on quasi-steady state schemes largely as a result of the narrower line profile in the lower temperature plasma. The inferred gain-narrowed linewidth of ~0.29 pm is also substantially narrower than previous measurements on quasi-steady state x-ray laser schemes. This study shows that the coherence of the x-ray laser beam can be improved by changing the laser pumping conditions. The x-ray laser is operating at 4 - 5 times the transform-limited pulse.
Compact soft x-ray laser sources are now used routinely for various applications primarily because of their high repetition rate, high photon fluence and short pulse duration characteristics. For some of these applications, for example interferometry of high density laser-produced plasmas, longer optical drive pulses, 6 - 13 ps (FWHM), have been implemented to maximize the x-ray output and coherence. It is therefore important to know the x-ray laser pulse length, shape and repeatability for these specific experiments as a baseline measurement but also to better understand the temporal behavior as a function of the pumping conditions in general. We report a detailed temporal characterization of the picosecond-driven 14.7 nm Ni-like Pd ion x-ray laser on the Compact Multipulse Terawatt (COMET) laser at LLNL using an ultrafast x-ray streak camera measurement of a horizontal slice of the near-field x-ray laser pattern. This is measured as a function of the chirped pulse amplification pumping laser conditions, including varying the pump pulse from 0.5 - 27 ps (FWHM), varying the plasma column length as well as investigating traveling wave (TW) and non-TW irradiation conditions.
We report on 2D near-field imaging experiments of the 11.9-nm Sn x-ray laser that were performed with a set of novel Mo/Y multilayer mirrors having reflectivities of up to 40% at normal and at 45° incidence. Second-moment analysis of the x-ray laser emission was used to determine values of the c-ray beam propagation factor M2 for a range of irradiation parameters. The results reveal a reduction of M2 with increasing prepulse intensity. The spatial size of the output is a factor of ~2 smaller than previously measured for the Pd x-ray laser, while the distance of the x-ray emission with respect to the target surface remains roughly the same.
We model recent experiments done using the COMET laser at Lawrence Livermore National Laboratory to illuminate slab targets of Pd up to 1.25 cm long with a two joule, 600 ps prepulse followed 700 psec later by a six joule, six psec drive pulse. The experiments measure the two-dimensional near-field and far-field laser patterns for the 14.7 nm Ni-like Pd x-ray laser line. The experiments are modeled using the LASNEX code to calculate the hydrodynamic evolution of the plasma and provide the temperatures and densities to the CRETIN code, which then does the kinetics calculations to determine the gain. Using a ray tracing code to simulate the near and far-field output the simulations are then compared with experiments. In addition we model recent experiments that used a streak camera to measure the time duration of the Pd X-ray laser when pumped with a constant energy short pulse with different time durations that ranged from 0.5 to 27 ps.
We present within this paper a series of experiments, which yield new observations to further our understanding of the transient collisional x-ray laser medium. We use the recently developed technique of picosecond x-ray laser interferometry to probe the plasma conditions in which the x-ray laser is generated and propagates. This yields two dimensional electron density maps of the plasma taken at different times relative to the peak of the 600ps plasma-forming beam. In another experimental campaign, the output of the x-ray laser plasma column is imaged with a spherical multilayer mirror onto a CCD camera to give a two-dimensional intensity map of the x-ray laser output. Near-field imaging gives insights into refraction, output intensity and spatial mode structure. Combining these images with the density maps gives an indication of the electron density at which the x-ray laser is being emitted at (yielding insights into the effect of density gradients on beam propagation). Experimental observations coupled with simulations predict that most effective coupling of laser pump energy occurs when the duration of the main heating pulse is comparable to the gain lifetime (~10ps for Ni-like schemes). This can increase the output intensity by more than an order of magnitude relative to the case were the same pumping energy is delivered within a shorter heating pulse duration (< 3ps). We have also conducted an experiment in which the output of the x-ray laser was imaged onto the entrance slit of a high temporal resolution streak camera. This effectively takes a one-dimensional slice of the x-ray laser spatial profile and sweeps it in time. Under some conditions we observe rapid movement of the x-ray laser (~ 3um/ps) towards the target surface.
During recent months we have continued investigations of many different aspects of x-ray lasers to characterize and improve the source and applications. This work has included temporal characterization of existing laser-heated x-ray lasers under a wide range of pumping conditions. We have also looked into more details at different applications of x-ray lasers among which was the interferometry of laser-produced and capillary discharge plasmas in several irradiation conditions for different target Z materials. The reduction of pump energy remains the most important for the generation of new compact x-ray lasers. Numerical studies show that there are some ways to improve several of the key parameters of x-ray lasers specifically repetition rates and efficiency.
In this work we demonstrate a soft x-ray laser with neon- like argon ions using a gas puff target irradiated with a combination of long 600 ps and short 6 ps high-power laser pulses with a total of 10 J energy. The gas puff target was formed by pulsed injection of gas from a high-pressure solenoid valve through a nozzle in the form of a narrow slit. The target was irradiated in a traveling-wave excitation geometry. Lasing was observed on the 3p 1S0 implies 3s 1P1 transition at 46.9 nm and the 3d 1P1 implies 3p 1P1 transition at 45.1 nm. Gain of 11 cm-1 was measured on these transitions for targets up to 0.9 cm long.
The development of the transient collisional excitation x-ray laser scheme using tabletop laser systems with multiple pulse capability has progressed rapidly in the last three years. The high small-signal gain and strong x-ray output have been demonstrated for laser drive energies of typically less than 10 J. We report recent x-ray laser experiments on the Lawrence Livermore National Laboratory (LLNL) Compact Multipulse Terawatt (COMET) tabletop facility using this technique. In particular, the saturated output from the Ni-like Pd ion 4d - 4p x-ray laser at 146.8 angstrom has been well characterized and has potential towards a useable x-ray source in a number of applications. One important application of a short wavelength x-ray laser beam with picosecond pulse duration is the study of a high density laser-produced plasma. We report the implementation of a Mach-Zehnder type interferometer using diffraction grating optics as beam splitters designed for the Ni-like Pd laser and show results from probing a 600 ps heated plasma. In addition, gas puff targets are investigated as an x-ray laser gain medium and we report results of strong lasing on the n equals 3 - 3 transitions of Ne-like Ar.
Experimental investigations on the conditions to achieve transient gain in neon-like Ti and nickel-like molybdenum XUV laser pumped by a 10-Hz sub-Joule femtosecond laser are presented. The 4d-4p (J equals 0-1) (lambda) equals 18.9 nm and 4f-4d (J equals 1-1) (lambda) equals 22.6 nm lines in Ni-like Mo as well as the 3p-3s (J equals 0-1) (lambda) equals 32.6-nm line in neon-like titanium have been observed. The Ni-like laser lines show a threshold behavior with respect to the pump irradiance as they appear only above 1015 W/cm2. Simulation for the fs-laser pumped Ni-like Mo XUV laser are also presented.
The technique of using a nsec pulse to preform and ionize the plasma followed by a psec pulse to heat the plasma has enabled low-Z nickel-like ions to achieve saturated output when driven by small lasers with less than ten joules of energy. We model experiments done using the COMET laser at LLNL and the P102 laser at Limeil to produce Ni-like Pd and Ag lasers. The COMET experiments use a 2 J, 600 ps prepulse followed 700 psec later by a 6 J, 6 psec drive pulse in a 1.6-cm long line focus. The P102 experiments used a somewhat larger energy and were able to use different combinations of frequency doubled light for both the prepulse and short pulse drive. The LASNEX code is used to calculate the hydrodynamic evolution of the plasma and provide the temperatures and densities to the CRETIN code, which then does the kinetics calculations to determine the gain. The temporal and spatial evolution of the plasmas are studied both with and without radiation transport included to understand the role of the self photopumping process on the gain of the Ni-like 4f implies 4D laser lines as well as the gain of the usual collisionally driven Ni-like 4d implies 4p laser lines. In particular we study why the 4f implies 4d line lases well only when frequency doubled light is used with the prepulse in the P102 experiments. Experimental results are presented for Ni-like Pd including two- dimensional near-field and far-field images.
We present experimental results of a high efficiency Ne-like Fe transient collisional excitation x-ray laser using the COMET 15 TW table-top laser system at LLNL. The plasma formation, ionization and collisional excitation of the x- ray laser have been optimized using two sequential laser pulses: a plasma formation beam with 5 J energy of 600 ps duration and a pump beam with 5 J energy of 1.2 ps duration. Since the observation of strong lasing on the 255 angstroms 3p - 3s J equals 0 - 1 transition of Ne-like Fe, we have achieved high gains of 35 cm-1 and saturation of the x-ray laser. A five-stage traveling wave excitation enhances the strongest Fe 3p - 3s 255 angstroms lasing line as well as additional x-ray lines. A careful characterization of the plasma column conditions using L-shell spectroscopy indicates the degree of ionization along the line focus.
Recently, the technique of using a nsec pulse to preform and ionize the plasma followed by a psec pulse to heat the plasma has enabled low-Z neon-like and nickel-like ions to lase driven by small lasers with only ten joules of energy. In this work we model recent experiments done using the COMET laser at LLNL to illuminate 1 cm long slab targets of Ti with a 4.8 J, 800 ps prepulse followed 1.6 nsec later by a 6 J, 1 psec drive pulse. The LASNEX code is used to calculate the hydrodynamic evolution of the plasma and provide the temperatures and densities of the XRASER code, which then does the kinetics calculations to determine the gain.
High resolution 2D imaging experiment on the saturated 18.9 nm Ni-like soft X-ray laser is presented. The imaging experiment allows measurement of the absolute output energy and intensity of the X-ray laser, while gives detailed information on the spatial characteristics of the X-ray laser for understanding the physics and further improving the performance of the X-ray laser.
Recent transient collisional excitation x-ray laser experiments are reported using the COMET tabletop laser driver at the Lawrence Livermore National Laboratory. Ne- like and Ni-like ion x-ray laser schemes have been investigated with a combination of long 600 ps and short approximately 1 ps high power laser pulses with 5 - 10 J total energy. We show small signal gain saturation for x-ray lasers when a reflection echelon traveling wave geometry is utilized. A gain length product of 18 has been achieved for the Ni-like Pd 4dyields4p J equals 0 - 1 line at 147 angstroms, with an estimated output of approximately 10 (mu) J. Strong lasing on the 119 angstroms Ni-like Sn line has also been observed. To our knowledge this is the first time gain saturation has been achieved on a tabletop laser driven scheme and is the shortest wavelength table-top x-ray laser demonstrated to date. In addition, we present preliminary results of the characterization of the line focus uniformity for a Ne-like ion scheme using L-shell spectroscopy.
This paper models recent experiments in which a solid titanium target was illuminated by several joules of combined energy from a nsec laser pulse to create a preplasma followed by a psec laser pulse to drive the gain. Gains greater than 200 cm-1 are predicted for the Ne-like Ti 3p 1S0 yields 3s 1P1 transition at 32.6 nm which is driven by the monopole collisional excitation. High gain is also predicted for the 3d 1P1 yields 3p 1P1 transition at 30.1 nm which is driven by a combination of collisional excitation and self photopumping. We also discuss the possibilities for driving a Ne-like Ge laser using this approach. For the Ni-like ions we model a solid molybdenum target under similar conditions used for Ti and predict gains greater than 300 cm-1 for the Ni-like Mo 4d 1S0 yields 4p 1P1 transition at 18.9 nm which is driven by the monopole collisional excitation. High gain is also predicted for a self photopumped 4f 1P1 yields 4d 1P1 transition at 22.0 nm and several other transitions driven by inner shell collisional ionization.
We discuss high resolution two-dimensional near-field images of the neon-like nickel and germanium x-ray laser obtained using the Asterix laser at the Max-Planck-Institute and the Nova laser at Lawrence Livermore National Laboratory. Our imaging diagnostic consisted of a concave multilayer mirror that imaged the output end of the x-ray laser line onto a backside illuminated x-ray CCD detector. A 25 micrometer thick wire positioned at the end of the target provided a spatial fiducial. With the Asterix iodine laser, a prepulse 5.23 ns before the main pulse, was used to irradiate slab targets. A great deal of structure was observed in the near field images, particularly in the J equals 0 - 1 emission. We observed a large difference in the spatial dependence of the J equals 0 - 1 and J equals 2 - 1 lines of germanium, with the J equals 2 - 1 emission peaking farther away from the original target surface. A larger prepulse moved the peak emission farther away from the target surface. For the Nova experiments we used a series of 100 ps pulses spaced 400 ps apart to illuminate a germanium target. We obtained high resolution images of both the J equals 0 - 1 and J equals 2 - 1 lines of Ge. these measurements are compared to hydrodynamic simulations coupled with atomic kinetics and including refraction effects.
We report the first demonstration of saturation in nickel-like x-ray lasers, specifically nickel-like Ag, In, Sn, and Sm x- ray lasers at wavelengths of 14, 12.6, 12.0 and 7.3 nm respectively. These x-ray lasers were found to be very monochromatic x-ray sources with the laser lines completely dominating the output spectra. Using high-resolution spatial imaging and angularly resolved streaking techniques, the output source sizes as well as the time histories, divergences, energies and spatial profiles of these x-ray lasers have been fully characterized. The output intensities of these x-ray lasers were measured to be in the range of 0.7 - 2 X 1011 W (DOT) cm-2 in approximately 40 ps. The high monochromaticity, narrow divergence, short pulse duration, high efficiency and high brightness of these x-ray lasers make them ideal candidates for many applications.
Recent studies of soft-x-ray and XUV lasers in Ne- and Ni-like ions using the Asterix IV iodine laser as a pump are reviewed. Progress achieved includes the observation of new laser lines in a number of low to medium-Z Ne-like ions at wavelengths from 20 to 87 nm, the reduction of the driver energy for neon- like S to a value of 20 J and lasing in Ni-like Sn at 12 nm. We also present recent results in characterizing near- and far-field patterns and compare them with predictions of simulations, using a 2D hydrodynamic code combined with a ray tracing code.
We present the first direct spatial measurement of the two dimensional gain profiles for a Ne-like ion using a slab target illuminated by the multiple pulse technique. To understand the spatial dependence of the gain in Ne-like Ge on the 19.6 nm laser line for plasmas driven by a series of 100 ps pulses 400 ps apart we did a series of Nova experiments backlighting short Ge amplifiers. Two-dimensional, high- resolution, spatial images of the 19.6 nm laser emission from the output aperture of the amplifiers were measured to determine the spatial position of the gain. The amplifier lengths were chosen to be short enough to avoid significant refraction of the beam. In previous imaging experiments which measured the near field output of the Ge laser, the position of the laser output was dominated by refraction effects. To assure good temporal overlap, we used the traveling wave geometry to illuminate both the amplifier and backlighter. The amplifier design included a wire fiducial which provided an absolute spatial reference and avoided the usual difficulty of determining the location of the target surface. We compare the measured gain with simulations done using LASNEX, which calculates the hydrodynamic evolution of the plasma, and XRASER, which uses the temperature and densities from LASNEX to do the gain and kinetics calculations.
A hot and dense plasma can be produced by high-power laser irradiation of a high-pressure gas puff target. The plasma emits strong x-ray radiation in low photon-energy range (soft x-rays and XUV radiation) and is considered to be used as a debrisless laser-produced x-ray source. It was shown that the laser-irradiated gas puff plasma is an ideal source for the high-resolution spectroscopic studies of complex spectra of the multicharged ions. This paper reports our investigations of x-ray spectra of heliumlike argon and neonlike krypton ions. The gas puff targets were created with the use of a specially designed high-pressure solenoid valve operating at a backing pressure up to 15 at and quipped with a sonic-type circular nozzle of 0.5 mm in diameter. Parameters of the gas puff targets were measured using x-ray shadowgraphy and laser interferometry. To irradiate the gas puff targets we have used a Nd:glass laser, which generates 10 J pulses in 1 ns FWHM. The laser beam was focused onto the gas puff target perpendicularly in respect to the flow of gas using an aspherical lens. The diameter of a laser beam in the focus were about 100 micrometers , what ensured the radiation power density to be of order of 1014 W/cm2. To measure x-ray spectra emitted by a laser-irradiated gas puff target we have used a simple focusing crystal spectrographs with a mica crystal curved into a spherical surface of radius R equals 100 mm. The spectra were recorded on Kodak RAR 2495 x-ray commercial film. The high resolving power of the spectrograph of about (lambda) /(Delta) (lambda) equals 10000 permitted high-precision wavelength spectral measurements. The measured x-ray spectra have the small spectra width of the observed lines associated with the low expansion velocity of the laser- irradiated gas puff plasma. Dielectronic sodiumlike satellites to neonlike krypton resonance lines have measured for the first time. High-resolution spectra of heliumlike argon were also obtained. The measured spectra have been used for diagnosing the plasma parameters.
We present results which show lasing at 79 angstrom in nickel-like neodymium (Z equals 60) when a series of short 100 - 150 ps pulses which are 400 - 500 ps apart are used to illuminate slab targets of neodymium. This multiple pulse technique was first used successfully with germanium and selenium targets where strong lasing was observed on the neon-like 3p yields 3s(J equals 0 yields 1) transitions at 196 and 182 angstrom, respectively. We also present results which use this technique on both higher and lower Z targets of neon-like ions. For the higher-Z ions such as yttrium, zirconium, and molybdenum we observe the usual lasing dominated by the pair of 3p yields 3s(J equals 2 yields 1) transitions as seen in other experiments using single pulse illumination. For lower-Z ions such as iron, nickel, and zinc we see dominant lasing from the 3p yields 3s(J equals 0 yields 1) transition however it is relatively weak for iron and increases with Z to become quite strong for zinc. We present results which show the advantages of coupled slab targets and of using a traveling wave geometry to drive targets with these short pulses. The main result of this work is combining the advantages of the double slab targets, the traveling wave geometry, and the multiple pulse technique to improve the output of the nickel-like neodymium laser at 70 angstrom.
This communication presents the results of wavelength calculations for neon-like ions to verify the resonance condition for a recently proposed x-ray laser scheme which is resonantly photopumped by Ly-(alpha) radiation from H-like Mg and which would lase on several 2p yields 2s transitions in Ne-like Ge. The energies of the excited and ground states were obtained using multiconfigurational Dirac-Fock (MCDF) method with the employment of different methods of the energy functional optimization. Particular attention has been given to the evaluation of the correlation corrections to the transition energies of neon-like ions within the combined MCDF+MZ approach, which uses the results of the MCDF calculations along with the Z-expansion data.
We are developing techniques to shorten the time duration of neon-like x-ray lasers while maintaining their high brightness in order to optimize their usefulness as a plasma diagnostic. Adjusting the duration of the pump laser pulse is shown to directly influence the duration of neon-like x-ray laser transitions. Using slab targets, multiple 100 ps pulses and traveling wave geometry we have shortened the duration of lasing transitions down to 45 ps for both the neon- like germanium and yttrium x-ray lasers. However for the neon-like yttrium laser the intensity of short duration pulses are down two orders of magnitude from the long duration pulses because of limitations of the driving laser. We are presently looking at curved targets and pulse shaping in order to more efficiently pump the Ne-like x-ray laser system and increase the output intensity of the lasing lines. The relative merits of using the germanium x-ray laser at 196 angstrom compared to the yttrium x-ray laser at 155 angstrom are discussed.
We have performed a systematic investigation of lasing on the neon-like 3p - 3s J equals 0 - 1 line in low-Z elements ranging from Cl to Ge using the prepulse technique. Laser pulses from the Asterix iodine laser (lambda equals 1.315 micrometers) were applied to slab targets with a low intensity prepulse 5 ns ahead of the main pulse. Prepulse energies ranged from 0.1% to 15% of the main pulse energy. In all materials lasing on the J equals 0 - 1 line was observed. In vanadium two J equals 0 - 1 lines were found to lase with approximately equal strength. The spatial position of lasing was determined for several materials and two prepulse levels. In addition, the sensitivity of lasing with respect to the mainpulse/prepulse ratio is reported.
We present results that show lasing on the 3p->3s (J = 0->1) transition in neon-like chromium (Z = 24), iron (Z = 26), and nickel (Z = 28) at 28.5, 25.5, and 23.1 nm, respectively. These results destroy the uniqueness of the lasing observed several years ago in neon-like titanium (Z = 22) at 32.6 nm on the same transition and makes highly unlikely the hypothesis that resonant photopumping is playing a significant role in the titanium laser. The titanium, chromium, iron, and nickel experiments all require a prepulse in order to lase, and our calculations suggest that the prepulse is an exciting new way to create a uniform low-density plasma that allows the proper conditions for gain and laser propagation for low-Zneon-like ions when illuminating a thick slab target. We also present an observation of hyperfine splitting in neon-like niobium at 14.6 nm and offer an explanation as to how the hyperfine effect is reducing the gain of neon-like ions with odd Z.
One method of improving the transverse spatial coherence of x-ray lasers (XRLs) is by adaptive spatial filtering of XRL apertures using geometric shaping in the form of bowtie or wedge XRLs. However, we must maintain the desired geometric shapes in exploding foil or slab configurations during the lasing period. As a first step toward understanding lasing in such geometries, we study the behavior of simple stripe XRLs. Past experience with stripe XRLs deposited on thick plastic substrates resulted in significantly weaker laser intensities as compared to line-focused slab XRLs. Possible reasons for this intensity reduction of stripe XRLs could include mixing at the laser boundary, and changes in plasma, kinetics, and hydrodynamic properties that affect laser gains and propagation. We present experimental and theoretical characterizations of germanium line-focused slab and stripe XRLs. Key experimental parameters we are studying include images of emission profiles of the laser blowoff, angular divergences, XRL output intensities, and ionization balances as we vary XRL designs. We compare the experimental results with 2-D laser deposition and hydrodynamics simulations using LASNEX, and study the changes in ionization balances and level populations from postprocessing LASNEX results.
We will present results which show lasing on the 3p yields 3s (J equals 0 yields 1) transition in neon-like chromium (Z equals 24), iron (Z equals 24), iron (Z equals 26), and nickel (Z equals 28) at 285, 255, and 231 angstroms respectively. This destroys the myth of titanium being unique and makes highly unlikely that the previously mentioned photo-pumping mechanism is playing a significant role in the titanium laser. The chromium, iron, and nickel experiments all require a prepulse in order to lase and our calculations suggest that the prepulse is an exciting new way to create a uniform low density plasma when illuminating a thick slab target. This allows the proper conditions for gain and laser propagation for low Z neon-like ions and may also be applicable to other systems such as low Z nickel-like ions. We also will present experiments done on other low-Z materials and offer an explanation as to how the hyperfine effect is destroying the gain of neon-like ions with odd Z.
Alan Wan, Juan Moreno, Brian MacGowan, Jeffrey Koch, Stephen Libby, Joseph Nilsen, Albert Osterheld, James Scofield, James Trebes, Bruno Van Wonterghem, Rosemary Walling
We will present experimental and theoretical characterizations of germanium line-focused and stripe x-ray lasers (XRLs). Key experimental parameters we will study include images of emission profiles of the laser blow-off, angular divergences, XRL output intensities, and ionization balances as we vary XRL designs. We will compare the experimental results with 2D laser deposition and hydrodynamics simulations using LASNEX, and study the changes in ionization balances and level populations from post-processing LASNEX results.
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