Validating and improving the global atmospheric transport model, therefore, requires precise measurement of the CO2 concentration profile. The differential absorption lidar (DIAL) is thought to be one of the best methods for observing the vertical distribution of greenhouse gases. One of its main advantages over other passive methods is its capacity for taking continuous measurements that provide high spatial and temporal resolutions of CO2. We had developed a ground based direct detection 1.6 μm DIAL to achieve measurements of vertical CO2 profiles. As the spectra of absorption lines of any molecules are influenced basically by the air temperature, it is important to measure the air temperature simultaneously. Then, we have improved the 1.6 μm DIAL system for simultaneous measurements of the CO2 concentration and temperature profiles in the lower-atmosphere. We conducted a field experiment to compare the new DIAL measurements with in situ sensor measurements. An open-path CO2 gas analyzer (LICOR. Inc., LI-7500) and temperature sensor (T&D TR-72Ui) were installed at the top of the building at a height of 42 m. The average difference in the CO2 concentration measured by the DIAL and LI-7500 was −0.01 ± 2.1 ppm. The average difference in the atmospheric temperature measured by the DIAL and TR-72Ui was −0.10 ± 0.28 °C. The new DIAL system is, therefore, capable of performing highly accurate vertical CO2 concentration and atmospheric temperature measurements.
We also conducted some continuous observations of CO2 concentration and temperature profiles in the lower atmosphere. In this paper, daily variation of CO2 concentration and temperature profiles are reported. We found that the accuracy of the CO2 concentration profiles measured with the new DIAL is improved significantly by the air temperature measurement.
This work was financially supported by the System Development Program for Advanced Measurement and Analysis of the Japan Science and Technology Agency.
In this paper, we propose a diode laser based differential absorption lidar (DIAL) for measuring lower-tropospheric water
vapor profile using the modulated pulse technique. The transmitter is based on single-mode diode laser and tapered
semiconductor optical amplifier with a peak power of 10W around 800nm absorption band, and the receiver telescope
diameter is 35cm. The selected wavelengths are compared to referenced wavelengths in terms of random error and
systematic errors. The key component of modulated pulse technique, a macropulse, is generated with a repetition rate of
10 kHz, and the modulation within the macropulse is coded according to a pseudorandom sequence with 100ns chip
width. As a result, we evaluate both single pulse modulation and pseudorandom coded pulse modulation technique. The
water vapor profiles conducted from these modulation techniques are compared to the real observation data in summer in
Japan.
The accurate vertical CO2 profiles in the troposphere are highly desirable in the inverse techniques to improve quantification and understanding of the global budget of CO2 and also global climate changes. Moreover, wind information is an important parameter for transport simulations and inverse estimation of surface CO2 flux. A differential absorption lidar (DIAL) is an attractive method for obtaining vertical CO2 profiles and we have developed an 1.6μm DIAL system to perform simultaneous measurements of CO2 concentration, atmospheric temperature profile and wind profile. The absorption cross sections of gas and air density depends on atmospheric temperature and pressure. Then precise temperature and pressure profiles are necessary for accurate CO2 mixing ratio measurement by DIAL. Laser beams of three wavelengths around a CO2 absorption line are transmitted alternately to the atmosphere for simultaneous measurements of CO2 concentration and temperature. The receiving optics include the near-infrared photomultiplier tube and a fiber Bragg grating (FBG) filter to detect a Doppler shift.
Inverse techniques using atmospheric transport models are developed to estimate the CO2 sources and sinks based on the
observed data. In comparison with the ground-based monitoring network, CO2 measurements for vertical profiles in the
troposphere have been due to the limited observations by using campaign-style aircrafts and the commercial airlines with
limited spatial and temporal coverage. The differential absorption lidar (DIAL) with the range resolution is expected to
bring several advantages over passive measurements, for example, daytime coverage and neglecting influences of
aerosol and cirrus layers. We have succeeded to develop the 1.6 μm DIAL technique using direct detection method for
measurement of CO2 concentration profiles in the atmosphere. This paper describes the advanced CO2 1.6 μm DIAL
technique consisting of the optical parametric generator (OPG) transmitter (10mJ/pulse) that excited by the LD pumped
Nd:YAG laser with high repetition rate (500Hz) and the receiving optics that included the large telescope with 60cm
diameter and the photomultiplier tube with high quantum efficiency (~8%) operating at the photon counting mode and
the narrowband interference filter (0.5nm bandwidth) for daytime observations. The CO2 concentration profiles from
ground to an altitude of 12km are conducted to measure with better than 1% standard deviation using 500m bins by this
CO2 DIAL.
We have constructed the lidar facility for survey of atmospheric structure over troposphere, stratosphere, mesosphere and low thermosphere over Kototabang (100.3E, 0.2S), Indonesia in the equatorial region. The lidar system consists of the Mie and Raman lidars for tropospheric aerosol, water vapor and cirrus cloud measurements, the Rayleigh lidar for stratospheric and mesospheric temperature measurements and the Resonance lidar for metallic species such as Na, Fe, Ca ion measurements and temperature measurements in the mesopause region. The laser system included in this lidar facility consists of three pulsed Nd:YAG lasers, a pulsed Ti:Sapphire laser seeded by a ring Ti:Sapphire laser and a dye laser. And, the receiving system consists of a Schmidt-Cassegrain telescope with 20cm diameter, a Schmidt-Cassegrain telescope with 35cm diameter and five Newtonian telescopes with 45cm diameter. The most parts of this lidar system are remotely controlled via the Internet from Tokyo Metropolitan University (TMU) in Japan.
The incoherent Doppler lidar technique using the frequency doubled Nd:YAG laser which was alternately tuned to the both slopes of one absorption line of the molecular iodine was developed and wind measurements were observed from 8 to 25km with 500m range resolution. Owing to the evaluation of measurement accuracy of this Doppler lidar, the truth of the zero wind is confirmed by using the direct reflection light from the hard target and the standard deviation is 0.35m/s. The comparison observations between the lidar wind velocities and the wind profiles of a wind profiler are performed experimentally.
We present a new method of the rotational Raman lidar using an absorption cell of metallic vapor. The conventional rotational Raman lidar can hardly measure the temperature profiles in the atmosphere containing a lot of aerosol particles like in the lower troposphere. In this paper, it is shown by the computer simulation that the aerosol scattering contamination disturbing the measurement can be easily eliminated by using a metallic vapor filter in addition to the interference filters. Moreover, the interference filters of which the characteristics affect decisively the measurement accuracy can be designed more suitably. We design and fabricate the lidar system with a Na vapor cell and a narrowband dye laser to prove the usefulness of this method experimentally.
We have developed the resonance scattering lidar system for measurements of mesospheric metallic species such as Na, K, Fe atoms and Ca ions and mesospheric temperature and wind. The flashlamp pumped Ti:sapphire laser injected by the seeder that consists of an external cavity laser diode is applied for measurements of the K and Fe atoms and the Ca ions. The sophisticated lidar system which consists of a pulsed dye oscillator and an amplifier system injection-seeded by a stabilized cw ring dye laser is also applied for Na atoms, temperature and wind measurements. Its injection-seeder consists of the single mode ring dye laser locked to the Na fluorescence line using the wavemeter and the Na vapor cell. The most characteristic of this laser system is to generate the comparatively high pulse energy ( more than 100mJ/pulse ) keeping up the narrow bandwidth ( about 0.1pm ). In this paper, the details of the laser design and the results observed by these lidar system are shown.
For the future spaceborne water vapor DIAL system, an airborne differential absorption lidar (DIAL) system in the near infrared has been developed. An injection seeded triple pulse Ti:sapphire laser is used for the transmitter and an LD pumped conductive-cooled Nd:YLF laser is employed for the pump laser of the Ti:sapphire laser. The entire system including the receiving telescope, receiving optics, an APD detector and signal processing system are developed. The system was onboard the Beechcraft B200 aircraft and flight tests of the system were conducted at three nights of November 1999.
A new incoherent Doppler lidar technique for atmospheric wind measurement is presented. This direct detection Doppler lidar is realized by the transmitting laser with two wavelengths and the receiving system with only one bandpass or absorption filter. We fabricated actually the Doppler lidar system using the frequency doubled Nd:YAG laser which was alternately tuned to the both slopes of one absorption line of the molecular iodine with an AO wavelength shifter, and performed simultaneous measurements of the eastward and northward wind components from 8 to 25km altitude with 500m vertical resolution. This Doppler lidar system is very useful to measure the wind profiles between lower troposphere and stratosphere by one effort.
Owing to understanding the transportation and chemical reaction of the aerosols, it is important to observe the aerosol density, depolarization ratio, wind profiles, temperature profiles and water vapor density simultaneously. We have prepared several lidar systems for simultaneous measurement of these constituents and parameters. The polarization lidar consists of the frequency-doubled Nd:YAG laser and polarizer for measurement of density and non-sphericity of the aerosol. The wind lidar consists of the incoherent Doppler lidar using the frequency-doubled Nd:YAG and the iodine vapor filter for measurement of the wind profiles. The temperature lidar is realized by the rotational Raman lidar with the Mie scatter blocking filter. And water vapor profiles are measured by a vibrational Raman lidar using the frequency doubled Nd:YAG laser. We got preliminary results of these parameters in the aerosol layer.
We have organized a network campaign for the observation of Asian dust in the spring of 1997 and 1998 in Japan. Through the communication with electric mail, we have successfully observed Kosa events by lidar, sunphotometer, and particle counter, etc. These data must be useful to analyze the transport mechanism of Asian dust and validate the satellite observations.
Characteristics of a flashlamp pumped Ti:sapphire laser seeded by an external cavity laser diode (ECLD) is reported. The ECLD consists of a commercially available laser diode, a diffraction grating and a tuning mirror. The laser diode does not have an anti-reflection coating. The tuning mirror is used to feed the first order diffraction beam back to the laser diode. The ECLD has the property of mode-hopping suppression that is useful for the laser radar applications. The linewidth (FWHM) of the ECLD is about 0.3 pm with an output power of 6 mW and the wavelength tuning range is 11 nm from 769 nm to 780 nm. Injection into the cavity of the Ti:sapphire laser is made through a polarizing prism located between a Ti:sapphire rod and a pockels cell. The linewidth (FWHM) of the flashlamp pumped Ti:sapphire laser injection seeded by the ECLD was about 0.55 pm consequently. This laser system is applied to observe the potassium layer in the mesopause region.
For future spaceborne water vapor DIAL systems, we started a laser design study in 1994. New laser materials such as Cr:LiSAF are very attractive, but at present there are no high power diode lasers for direct pumping those materials. Therefore we determined to develop a high power diode-pumped Nd:YLF laser and Ti:sapphire laser for water vapor DIAL. The output energy of Nd:YLF laser is expected to be 550 mJ at 1053 nm and 400 mJ at 527 nm with a maximum repetition rate of 150 Hz. A Ti:sapphire laser will be pumped by the SHG of the Nd:YLF laser. Tuning of the Ti:sapphire laser to a strong absorption line (ON1), a weak absorption line (ON2) of water vapor and an off line (OFF) is made by an injection seeder which consists of two single longitudinal mode laser diode modules. Two on-line laser diodes are locked to water vapor absorption lines using an absorption cell or a photo-acoustic cell. These three laser lines (ON1, OFF and ON2) are transmitted into the atmosphere with a triple pulse technique for measurements of water vapor profiles from the ground up to 10 km. The laser spectral width of the on line is expected to be 0.5 pm with a stability of 0.05 pm. The output energy of each laser line is to be more than 100 mJ. This laser system will be developed within three years, and then incorporated as an airborne water DIAL.
This paper presents the results of computer simulation associated with differential absorption lidar (DIAL) measurements of atmospheric water vapor profiles from spaceborne for the low- latitude (15N), for summer and winter in the mid-latitude (45N), and for summer and winter in the high-latitude (60N), respectively. We think that a Nd:YAG laser pumped Ti:sapphire laser is available to use with the spaceborne water vapor lidar at present. Then the water vapor absorption lines used in these calculations are in the 820 nm spectral region. The analysis suggests that the spaceborne DIAL system needs 2 or 3 pairs of the on (strong absorption) - off (weak absorption) laser lines for less than 10% profile measurements accuracy from 0 km altitude to about 10 km altitude in the mid-latitude.
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