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Plasmonic transdimensional materials offer advances such as thickness-controlled light-matter coupling and novel space-time symmetry breaking phenomena to further develop the fields of nanophotonics and optical metasurfaces. Much is unclear though about their optical response and quantum near-field effects. We use quantum electrodynamics and a confinement-induced nonlocal dielectric response model to study the epsilon-near-zero modes of metallic films in the transdimensional regime. New remarkable effects are revealed such as the plasmon mode degeneracy lifting and the dipole emitter coupling to the split epsilon-near-zero modes, leading to thickness-controlled dipolar spontaneous emission with up to three-orders-of-magnitude increased rates.
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Igor Bondarev, Hamze Mousavi, Vlad Shalaev, "Transdimensional epsilon-near-zero modes in planar plasmonic nanostructures," Proc. SPIE 11461, Active Photonic Platforms XII, 114611I (20 August 2020); https://doi.org/10.1117/12.2567241