The control of optical properties by electric means is the key to optoelectronic applications. For atomically thin two-dimensional (2D) materials, the natural advantage lies in that the carrier doping could be readily controlled through the electric gating effect, possibly affecting the optical properties. By exploiting this advantage, we studied nonlinear optical responses from doped graphene, including both coherent nonlinear processes such as the second harmonic generation (SHG) and third harmonic generation (THG), and the incoherent ultrafast photoluminescence (PL). The demonstration of these broadband, electrically tunable nonlinear optical responses in graphene is promising for a host of nonlinear optical applications.
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