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In this work, we study the enhanced nonlinear light-matter interaction in hybrid Weyl-semimetal-plasmonic structure by depositing silver nanocubes on a TaAs surface with a silicon nitride spacer thus leveraging the unique ability of plasmonics to squeeze electromagnetic field within a small volume far below the diffraction limit. Pumping the fabricated hybrid structure utilizing a 800-nm fundamental wavelength pulse at 100 fs we achieve second harmonic generation (SHG) at 400 nm with a 300 percent enhancement of SHG signal while the estimated actual plasmonic SHG enhancement is 90-fold.
Alexandra Boltasseva
"Plasmonically enhanced second harmonic generation in TaAs Weyl semimetal (Conference Presentation)", Proc. SPIE PC12195, Metamaterials, Metadevices, and Metasystems 2022, PC121950R (3 October 2022); https://doi.org/10.1117/12.2633224
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Alexandra Boltasseva, "Plasmonically enhanced second harmonic generation in TaAs Weyl semimetal (Conference Presentation)," Proc. SPIE PC12195, Metamaterials, Metadevices, and Metasystems 2022, PC121950R (3 October 2022); https://doi.org/10.1117/12.2633224