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We investigated THz phonon-polaritons by incorporating virtually free-standing lead halide perovskite into Fabry-Perot cavities. Rabi splitting occurred when the cavity resonance is in tune with the phonon resonance due to the strong coupling between the resonances. The Rabi splitting increased with the perovskite thickness, reaching 2.4 times of the strong coupling criterion; clear quantum beat oscillations were observed in the time domain. We also fabricated the flexible polariton devices using a plastic substrate for the development of tunable quantum states, controllable with mechanical bending processes.
Hwan Sik Kim,Abbas Ahmad Khan, andYeong-Hwan Ahn
"Enhanced coupling between lead halide perovskite phonons and THz fields in a flexible Fabry-Perot cavity", Proc. SPIE PC12419, Ultrafast Phenomena and Nanophotonics XXVII, (15 March 2023); https://doi.org/10.1117/12.2649709
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Hwan Sik Kim, Abbas Ahmad Khan, Yeong-Hwan Ahn, "Enhanced coupling between lead halide perovskite phonons and THz fields in a flexible Fabry-Perot cavity," Proc. SPIE PC12419, Ultrafast Phenomena and Nanophotonics XXVII, (15 March 2023); https://doi.org/10.1117/12.2649709